Comparing two synthesis methods: Exploring unique characteristics and catalytic activity of fenton catalyst Fe3O4/zeolite-NaY in methylene blue degradation

Dinia Astira; Romario Abdullah; Utari Zulfiani; Dety Oktavia Sulistiono; Zeni Rahmawati; Triyanda Gunawan; Mohd Hafiz Dzarfan Othman; Muhammad Hasan; Ratna Ediati; Hamzah Fansuri

doi:10.1016/j.cscee.2024.100963

Comparing two synthesis methods: Exploring unique characteristics and catalytic activity of fenton catalyst Fe₃O₄/zeolite-NaY in methylene blue degradation

Dinia Astira, Romario Abdullah, Utari Zulfiani, Dety Oktavia Sulistiono, Zeni Rahmawati, Triyanda Gunawan, Mohd Hafiz Dzarfan Othman, Muhammad Hasan, Ratna Ediati, Hamzah Fansuri^*

^*Corresponding author for this work

Research output: Contribution to journal › Article › peer-review

Abstract

A composite catalyst was developed to degrade methylene blue (MB) via the Fenton reaction from Fe₃O₄ and H₂O₂ with zeolite-NaY as magnetite support to reduce agglomeration. Hydrothermal and co-precipitation approaches were used to synthesize the composite. The co-precipitation method here was proven to be more suitable to produce the composite. Under optimal conditions, all composite catalysts achieved a remarkable MB reduction (more than 90 %) as confirmed through TLC analysis and UV–Vis spectra. Notably, based on linear regression, FeZ-A maintained over 60 % activity after 15 uses, while FeZ-2 showed the least Fe ion leaching. This demonstrated the effectiveness and stability of the developed catalysts.

Original language	English
Article number	100963
Journal	Case Studies in Chemical and Environmental Engineering
Volume	10
DOIs	https://doi.org/10.1016/j.cscee.2024.100963
Publication status	Published - Dec 2024

Keywords

Catalyst
Composite
FeO
Hetero-fenton
Wastewater treatment
Zeolite-NaY

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10.1016/j.cscee.2024.100963

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Astira, D., Abdullah, R., Zulfiani, U., Sulistiono, D. O., Rahmawati, Z., Gunawan, T., Dzarfan Othman, M. H., Hasan, M., Ediati, R., & Fansuri, H. (2024). Comparing two synthesis methods: Exploring unique characteristics and catalytic activity of fenton catalyst Fe₃O₄/zeolite-NaY in methylene blue degradation. Case Studies in Chemical and Environmental Engineering, 10, Article 100963. https://doi.org/10.1016/j.cscee.2024.100963

@article{b505a2c2978e4fbfa6fb5cce138e91af,

title = "Comparing two synthesis methods: Exploring unique characteristics and catalytic activity of fenton catalyst Fe3O4/zeolite-NaY in methylene blue degradation",

abstract = "A composite catalyst was developed to degrade methylene blue (MB) via the Fenton reaction from Fe3O4 and H2O2 with zeolite-NaY as magnetite support to reduce agglomeration. Hydrothermal and co-precipitation approaches were used to synthesize the composite. The co-precipitation method here was proven to be more suitable to produce the composite. Under optimal conditions, all composite catalysts achieved a remarkable MB reduction (more than 90 %) as confirmed through TLC analysis and UV–Vis spectra. Notably, based on linear regression, FeZ-A maintained over 60 % activity after 15 uses, while FeZ-2 showed the least Fe ion leaching. This demonstrated the effectiveness and stability of the developed catalysts.",

keywords = "Catalyst, Composite, FeO, Hetero-fenton, Wastewater treatment, Zeolite-NaY",

author = "Dinia Astira and Romario Abdullah and Utari Zulfiani and Sulistiono, {Dety Oktavia} and Zeni Rahmawati and Triyanda Gunawan and {Dzarfan Othman}, {Mohd Hafiz} and Muhammad Hasan and Ratna Ediati and Hamzah Fansuri",

note = "Publisher Copyright: {\textcopyright} 2024 The Authors",

year = "2024",

month = dec,

doi = "10.1016/j.cscee.2024.100963",

language = "English",

volume = "10",

journal = "Case Studies in Chemical and Environmental Engineering",

issn = "2666-0164",

publisher = "Elsevier Ltd.",

}

Astira, D, Abdullah, R, Zulfiani, U, Sulistiono, DO, Rahmawati, Z, Gunawan, T, Dzarfan Othman, MH, Hasan, M, Ediati, R & Fansuri, H 2024, 'Comparing two synthesis methods: Exploring unique characteristics and catalytic activity of fenton catalyst Fe₃O₄/zeolite-NaY in methylene blue degradation', Case Studies in Chemical and Environmental Engineering, vol. 10, 100963. https://doi.org/10.1016/j.cscee.2024.100963

TY - JOUR

T1 - Comparing two synthesis methods

T2 - Exploring unique characteristics and catalytic activity of fenton catalyst Fe3O4/zeolite-NaY in methylene blue degradation

AU - Astira, Dinia

AU - Abdullah, Romario

AU - Zulfiani, Utari

AU - Sulistiono, Dety Oktavia

AU - Rahmawati, Zeni

AU - Gunawan, Triyanda

AU - Dzarfan Othman, Mohd Hafiz

AU - Hasan, Muhammad

AU - Ediati, Ratna

AU - Fansuri, Hamzah

PY - 2024/12

Y1 - 2024/12

N2 - A composite catalyst was developed to degrade methylene blue (MB) via the Fenton reaction from Fe3O4 and H2O2 with zeolite-NaY as magnetite support to reduce agglomeration. Hydrothermal and co-precipitation approaches were used to synthesize the composite. The co-precipitation method here was proven to be more suitable to produce the composite. Under optimal conditions, all composite catalysts achieved a remarkable MB reduction (more than 90 %) as confirmed through TLC analysis and UV–Vis spectra. Notably, based on linear regression, FeZ-A maintained over 60 % activity after 15 uses, while FeZ-2 showed the least Fe ion leaching. This demonstrated the effectiveness and stability of the developed catalysts.

AB - A composite catalyst was developed to degrade methylene blue (MB) via the Fenton reaction from Fe3O4 and H2O2 with zeolite-NaY as magnetite support to reduce agglomeration. Hydrothermal and co-precipitation approaches were used to synthesize the composite. The co-precipitation method here was proven to be more suitable to produce the composite. Under optimal conditions, all composite catalysts achieved a remarkable MB reduction (more than 90 %) as confirmed through TLC analysis and UV–Vis spectra. Notably, based on linear regression, FeZ-A maintained over 60 % activity after 15 uses, while FeZ-2 showed the least Fe ion leaching. This demonstrated the effectiveness and stability of the developed catalysts.

KW - Catalyst

KW - Composite

KW - FeO

KW - Hetero-fenton

KW - Wastewater treatment

KW - Zeolite-NaY

UR - http://www.scopus.com/inward/record.url?scp=85205004166&partnerID=8YFLogxK

U2 - 10.1016/j.cscee.2024.100963

DO - 10.1016/j.cscee.2024.100963

M3 - Article

AN - SCOPUS:85205004166

SN - 2666-0164

VL - 10

JO - Case Studies in Chemical and Environmental Engineering

JF - Case Studies in Chemical and Environmental Engineering

M1 - 100963

ER -

Comparing two synthesis methods: Exploring unique characteristics and catalytic activity of fenton catalyst Fe₃O₄/zeolite-NaY in methylene blue degradation

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Comparing two synthesis methods: Exploring unique characteristics and catalytic activity of fenton catalyst Fe3O4/zeolite-NaY in methylene blue degradation

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Keywords

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Recent Findings from Institut Teknologi Sepuluh Nopember Highlight Research in Environmental Engineering (Comparing two synthesis methods: Exploring unique characteristics and catalytic activity of fenton catalyst Fe3O4/zeolite-NaY in methylene ...)

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Comparing two synthesis methods: Exploring unique characteristics and catalytic activity of fenton catalyst Fe₃O₄/zeolite-NaY in methylene blue degradation