Efficient degradation of methyl orange through photo-Fenton processes with MIL-100(Fe) modified Fe3O4 (Fe3O4@MIL-100(Fe)) catalyst

Melani Puji Puspitasari; Jeesica Hermayanti Pratama; Roshid Adi Nugroho; Witri Wahyu Lestari; Yusnadia Kemala; Teguh Endah Saraswati; Hamzah Fansuri; Rino Rakhmata Mukti; Rujito S.R. Suharbiansah

doi:10.21924/cst.9.2.2024.1493

Efficient degradation of methyl orange through photo-Fenton processes with MIL-100(Fe) modified Fe₃O₄ (Fe₃O₄@MIL-100(Fe)) catalyst

Melani Puji Puspitasari
, Jeesica Hermayanti Pratama
, Roshid Adi Nugroho
, Witri Wahyu Lestari^*
, Yusnadia Kemala
, Teguh Endah Saraswati
, Hamzah Fansuri
, Rino Rakhmata Mukti
, Rujito S.R. Suharbiansah

^*Corresponding author for this work

Universitas Sebelas Maret
Institut Teknologi Sepuluh Nopember
Bandung Institute of Technology
Leipzig University

Research output: Contribution to journal › Article › peer-review

4 Citations (Scopus)

Abstract

The research successfully synthesized a composite MIL-100(Fe) modified Fe3O4 (Fe3O4@MIL-100(Fe)) catalyst and examined its efficiency in degrading methyl orange (MO) through the photo-Fenton process compared to Fenton. The different percentages of Fe3O4 were integrated into MIL-100(Fe) and their effects on material characteristics and degradation capabilities were studied. Ex-situ synthesis involved varying Fe3O4 weight ratios (3, 10, and 20% w/w). Characterization techniques confirmed the integration of Fe3O4 and MIL-100(Fe) and revealed changes in surface area, pore size, and thermal stability with Fe3O4 addition. Meanwhile, removal tests showed promising results with the photo-Fenton process exhibiting maximum efficiency (95.51%) using 10% Fe3O4@MIL-100(Fe). This study provides valuable insights into developing efficient photo-Fenton catalysts for environmental remediation, particularly for addressing dye pollution in wastewater by highlighting the potential of Fe3O4@MIL-100(Fe) composites in this context.

Original language	English
Pages (from-to)	252-261
Number of pages	10
Journal	Communications in Science and Technology
Volume	9
Issue number	2
DOIs	https://doi.org/10.21924/cst.9.2.2024.1493
Publication status	Published - 2024

Keywords

Fe3O4
Fenton
MIL-100(Fe)
methyl orange
photo-Fenton

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10.21924/cst.9.2.2024.1493

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Puspitasari, M. P., Pratama, J. H., Nugroho, R. A., Lestari, W. W., Kemala, Y., Saraswati, T. E., Fansuri, H., Mukti, R. R., & Suharbiansah, R. S. R. (2024). Efficient degradation of methyl orange through photo-Fenton processes with MIL-100(Fe) modified Fe₃O₄ (Fe₃O₄@MIL-100(Fe)) catalyst. Communications in Science and Technology, 9(2), 252-261. https://doi.org/10.21924/cst.9.2.2024.1493

@article{a2b88bcf72e94f1084174c8b97e3a7a7,

title = "Efficient degradation of methyl orange through photo-Fenton processes with MIL-100(Fe) modified Fe3O4 (Fe3O4@MIL-100(Fe)) catalyst",

abstract = "The research successfully synthesized a composite MIL-100(Fe) modified Fe3O4 (Fe3O4@MIL-100(Fe)) catalyst and examined its efficiency in degrading methyl orange (MO) through the photo-Fenton process compared to Fenton. The different percentages of Fe3O4 were integrated into MIL-100(Fe) and their effects on material characteristics and degradation capabilities were studied. Ex-situ synthesis involved varying Fe3O4 weight ratios (3, 10, and 20\% w/w). Characterization techniques confirmed the integration of Fe3O4 and MIL-100(Fe) and revealed changes in surface area, pore size, and thermal stability with Fe3O4 addition. Meanwhile, removal tests showed promising results with the photo-Fenton process exhibiting maximum efficiency (95.51\%) using 10\% Fe3O4@MIL-100(Fe). This study provides valuable insights into developing efficient photo-Fenton catalysts for environmental remediation, particularly for addressing dye pollution in wastewater by highlighting the potential of Fe3O4@MIL-100(Fe) composites in this context.",

keywords = "Fe3O4, Fenton, MIL-100(Fe), methyl orange, photo-Fenton",

author = "Puspitasari, \{Melani Puji\} and Pratama, \{Jeesica Hermayanti\} and Nugroho, \{Roshid Adi\} and Lestari, \{Witri Wahyu\} and Yusnadia Kemala and Saraswati, \{Teguh Endah\} and Hamzah Fansuri and Mukti, \{Rino Rakhmata\} and Suharbiansah, \{Rujito S.R.\}",

year = "2024",

doi = "10.21924/cst.9.2.2024.1493",

language = "English",

volume = "9",

pages = "252--261",

journal = "Communications in Science and Technology",

issn = "2502-9258",

publisher = "Komunitas Ilmuwan dan Profesional Muslim Indonesia",

number = "2",

}

Puspitasari, MP, Pratama, JH, Nugroho, RA, Lestari, WW, Kemala, Y, Saraswati, TE, Fansuri, H, Mukti, RR & Suharbiansah, RSR 2024, 'Efficient degradation of methyl orange through photo-Fenton processes with MIL-100(Fe) modified Fe₃O₄ (Fe₃O₄@MIL-100(Fe)) catalyst', Communications in Science and Technology, vol. 9, no. 2, pp. 252-261. https://doi.org/10.21924/cst.9.2.2024.1493

TY - JOUR

T1 - Efficient degradation of methyl orange through photo-Fenton processes with MIL-100(Fe) modified Fe3O4 (Fe3O4@MIL-100(Fe)) catalyst

AU - Puspitasari, Melani Puji

AU - Pratama, Jeesica Hermayanti

AU - Nugroho, Roshid Adi

AU - Lestari, Witri Wahyu

AU - Kemala, Yusnadia

AU - Saraswati, Teguh Endah

AU - Fansuri, Hamzah

AU - Mukti, Rino Rakhmata

AU - Suharbiansah, Rujito S.R.

PY - 2024

Y1 - 2024

N2 - The research successfully synthesized a composite MIL-100(Fe) modified Fe3O4 (Fe3O4@MIL-100(Fe)) catalyst and examined its efficiency in degrading methyl orange (MO) through the photo-Fenton process compared to Fenton. The different percentages of Fe3O4 were integrated into MIL-100(Fe) and their effects on material characteristics and degradation capabilities were studied. Ex-situ synthesis involved varying Fe3O4 weight ratios (3, 10, and 20% w/w). Characterization techniques confirmed the integration of Fe3O4 and MIL-100(Fe) and revealed changes in surface area, pore size, and thermal stability with Fe3O4 addition. Meanwhile, removal tests showed promising results with the photo-Fenton process exhibiting maximum efficiency (95.51%) using 10% Fe3O4@MIL-100(Fe). This study provides valuable insights into developing efficient photo-Fenton catalysts for environmental remediation, particularly for addressing dye pollution in wastewater by highlighting the potential of Fe3O4@MIL-100(Fe) composites in this context.

AB - The research successfully synthesized a composite MIL-100(Fe) modified Fe3O4 (Fe3O4@MIL-100(Fe)) catalyst and examined its efficiency in degrading methyl orange (MO) through the photo-Fenton process compared to Fenton. The different percentages of Fe3O4 were integrated into MIL-100(Fe) and their effects on material characteristics and degradation capabilities were studied. Ex-situ synthesis involved varying Fe3O4 weight ratios (3, 10, and 20% w/w). Characterization techniques confirmed the integration of Fe3O4 and MIL-100(Fe) and revealed changes in surface area, pore size, and thermal stability with Fe3O4 addition. Meanwhile, removal tests showed promising results with the photo-Fenton process exhibiting maximum efficiency (95.51%) using 10% Fe3O4@MIL-100(Fe). This study provides valuable insights into developing efficient photo-Fenton catalysts for environmental remediation, particularly for addressing dye pollution in wastewater by highlighting the potential of Fe3O4@MIL-100(Fe) composites in this context.

KW - Fe3O4

KW - Fenton

KW - MIL-100(Fe)

KW - methyl orange

KW - photo-Fenton

UR - https://www.scopus.com/pages/publications/85213962462

U2 - 10.21924/cst.9.2.2024.1493

DO - 10.21924/cst.9.2.2024.1493

M3 - Article

AN - SCOPUS:85213962462

SN - 2502-9258

VL - 9

SP - 252

EP - 261

JO - Communications in Science and Technology

JF - Communications in Science and Technology

IS - 2

ER -

Efficient degradation of methyl orange through photo-Fenton processes with MIL-100(Fe) modified Fe₃O₄ (Fe₃O₄@MIL-100(Fe)) catalyst

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Keywords

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